Bailundo is a municipality, with a population of 294,494, and a town, with a population of 70,481, in the province of Huambo, Angola. In the 1990…Bailundo is a municipality, with a population of 294,494, and a town, with a population of 70,481, in the province of Huambo, Angola. In the 1990s, Bailundo was the location of the headquarters of UNITA leader Jonas Savimbi.